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    Nanostructure of Calcium Silicate Hydrates in Cements

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    Type
    Article
    Authors
    Skinner, L. B.
    Chae, S. R.
    Benmore, C. J.
    Wenk, H. R.
    Monteiro, P. J. M.
    KAUST Grant Number
    KUS-11-004021
    Date
    2010-05-11
    Permanent link to this record
    http://hdl.handle.net/10754/598952
    
    Metadata
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    Abstract
    Calcium silicate hydrate (CSH) is the major volume phase in the matrix of Portland cement concrete. Total x-ray scattering measurements with synchrotron x rays on synthetic CSH(I) shows nanocrystalline ordering with a particle diameter of 3.5(5) nm, similar to a size-broadened 1.1 nm tobermorite crystal structure. The CSH component in hydrated tricalcium silicate is found to be similar to CSH(I). Only a slight bend and additional disorder within the CaO sheets is required to explain its nanocrystalline structure. © 2010 The American Physical Society.
    Citation
    Skinner LB, Chae SR, Benmore CJ, Wenk HR, Monteiro PJM (2010) Nanostructure of Calcium Silicate Hydrates in Cements. Physical Review Letters 104. Available: http://dx.doi.org/10.1103/PhysRevLett.104.195502.
    Sponsors
    This publication was based on work supported in part by Grant No. KUS-11-004021, made by King Abdullah University of Science and Technology (KAUST). This work was supported by the U.S. DOE, Argonne National Laboratory under Contract No. DE-AC02-06CH11357. Also, thanks to Dr. Simon Clark, Dr. Juyoung Ha, Cagla Meral, and Elizabeth Mannering for their help with the production of this paper; and to Gordon Chan and Dr. Laila Raki for their help with the sample synthesis.
    Publisher
    American Physical Society (APS)
    Journal
    Physical Review Letters
    DOI
    10.1103/PhysRevLett.104.195502
    PubMed ID
    20866975
    ae974a485f413a2113503eed53cd6c53
    10.1103/PhysRevLett.104.195502
    Scopus Count
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