Thon, Susanna M.
Adachi, Michael M.
Labelle, André J.
Sargent, Edward H.
KAUST Grant NumberKUS-11-009-21
Online Publication Date2013-03-06
Print Publication Date2013-04-10
Permanent link to this recordhttp://hdl.handle.net/10754/598684
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AbstractRecent advances in spectrally tuned, solution-processed plasmonic nanoparticles have provided unprecedented control over light's propagation and absorption via engineering at the nanoscale. Simultaneous parallel progress in colloidal quantum dot photovoltaics offers the potential for low-cost, large-area solar power; however, these devices suffer from poor quantum efficiency in the more weakly absorbed infrared portion of the sun's spectrum. Here, we report a plasmonic-excitonic solar cell that combines two classes of solution-processed infrared materials that we tune jointly. We show through experiment and theory that a plasmonic-excitonic design using gold nanoshells with optimized single particle scattering-to-absorption cross-section ratios leads to a strong enhancement in near-field absorption and a resultant 35% enhancement in photocurrent in the performance-limiting near-infrared spectral region. © 2013 American Chemical Society.
CitationPaz-Soldan D, Lee A, Thon SM, Adachi MM, Dong H, et al. (2013) Jointly Tuned Plasmonic–Excitonic Photovoltaics Using Nanoshells. Nano Lett 13: 1502–1508. Available: http://dx.doi.org/10.1021/nl304604y.
SponsorsThis publication is based in part on work supported by an award (KUS-11-009-21) from the King Abdullah University of Science and Technology (KAUST), by the Ontario Research Fund Research Excellence Program and by the Natural Sciences and Engineering Research Council (NSERC) of Canada. The authors thank I. Kramer, E. Palmiano, R. Wolowiec and D. Kopilovic for their help during the course of the study. H.D. would like to acknowledge financial support from China Scholarship Council (CSC).
PublisherAmerican Chemical Society (ACS)
CollectionsPublications Acknowledging KAUST Support
- Infrared colloidal quantum dots for photovoltaics: fundamentals and recent progress.
- Authors: Tang J, Sargent EH
- Issue date: 2011 Jan 4
- Depleted-heterojunction colloidal quantum dot solar cells.
- Authors: Pattantyus-Abraham AG, Kramer IJ, Barkhouse AR, Wang X, Konstantatos G, Debnath R, Levina L, Raabe I, Nazeeruddin MK, Grätzel M, Sargent EH
- Issue date: 2010 Jun 22
- Efficient, stable infrared photovoltaics based on solution-cast colloidal quantum dots.
- Authors: Koleilat GI, Levina L, Shukla H, Myrskog SH, Hinds S, Pattantyus-Abraham AG, Sargent EH
- Issue date: 2008 May
- The donor-supply electrode enhances performance in colloidal quantum dot solar cells.
- Authors: Maraghechi P, Labelle AJ, Kirmani AR, Lan X, Adachi MM, Thon SM, Hoogland S, Lee A, Ning Z, Fischer A, Amassian A, Sargent EH
- Issue date: 2013 Jul 23
- Efficient spray-coated colloidal quantum dot solar cells.
- Authors: Kramer IJ, Minor JC, Moreno-Bautista G, Rollny L, Kanjanaboos P, Kopilovic D, Thon SM, Carey GH, Chou KW, Zhitomirsky D, Amassian A, Sargent EH
- Issue date: 2015 Jan 7