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    Carbon dioxide assist for non-aqueous sodium–oxygen batteries

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    Type
    Article
    Authors
    Das, Shyamal K.
    Xu, Shaomao
    Archer, Lynden A. cc
    KAUST Grant Number
    KUS-C1-018-02
    Date
    2013-02
    Permanent link to this record
    http://hdl.handle.net/10754/597727
    
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    Abstract
    We report a novel non-aqueous Na-air battery that utilizes a gas mixture of CO2 and O2. The battery exhibits a high specific energy of 6500-7000 Whkg- 1 (based on the carbon mass) over a range of CO2 feed compositions. The energy density achieved is higher, by 200% to 300%, than that obtained in pure oxygen. Ex-situ FTIR and XRD analysis reveal that Na2O2, Na2C2O 4 and Na2CO3 are the principal discharge products. The Na-CO2/O2 and Mg-CO2/O 2 battery platforms provide a promising, new approach for CO 2 capture and generation of electrical energy. © 2012 Elsevier B.V. All rights reserved.
    Citation
    Das SK, Xu S, Archer LA (2013) Carbon dioxide assist for non-aqueous sodium–oxygen batteries. Electrochemistry Communications 27: 59–62. Available: http://dx.doi.org/10.1016/j.elecom.2012.10.036.
    Sponsors
    This work was supported in part by Energy Materials Center at Cornell (award no. DE-SC0001086), and by award no. KUS-C1-018-02 made through King Abdullah University of Science and Technology (KAUST).
    Publisher
    Elsevier BV
    Journal
    Electrochemistry Communications
    DOI
    10.1016/j.elecom.2012.10.036
    ae974a485f413a2113503eed53cd6c53
    10.1016/j.elecom.2012.10.036
    Scopus Count
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