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    Materials Meets Concepts in Molecule-Based Electronics

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    Type
    Article
    Authors
    Ortmann, Frank
    Radke, K. Sebastian
    Günther, Alrun
    Kasemann, Daniel
    Leo, Karl
    Cuniberti, Gianaurelio
    KAUST Department
    KAUST Solar Center (KSC)
    Physical Science and Engineering (PSE) Division
    Date
    2014-10-14
    Online Publication Date
    2014-10-14
    Print Publication Date
    2015-04
    Permanent link to this record
    http://hdl.handle.net/10754/594142
    
    Metadata
    Show full item record
    Abstract
    In this contribution, molecular materials are highlighted as an important topic in the diverse field of condensed matter physics, with focus on their particular electronic and transport properties. A better understanding of their performance in various applications and devices demands for an extension of basic theoretical approaches to describe charge transport in molecular materials, including the accurate description of electron-phonon coupling. Starting with the simplest case of a molecular junction and moving on to larger aggregates of bulk organic semiconductors, charge-transport regimes from ballistic motion to incoherent hopping, which are frequently encountered in molecular systems under respective conditions, are discussed. Transport features of specific materials are described through ab initio material parameters whose determination is addressed. © 2014 Wiley-VCH Verlag GmbH & Co. KGaA.
    Citation
    Ortmann F, Radke KS, Günther A, Kasemann D, Leo K, et al. (2014) Materials Meets Concepts in Molecule-Based Electronics. Advanced Functional Materials 25: 1933–1954. Available: http://dx.doi.org/10.1002/adfm.201402334.
    Sponsors
    This work is partly based on original research of H. Kleemann, D. Nozaki, and K. Hannewald. The authors gratefully acknowledge fruitful discussions with all of them. F.O. would like to thank the DFG for financial support within the Emmy-Noether funding scheme and A.G. thanks the Dr. Isolde-Dietrich-Stiftung for its financial support. This work was partly supported by the DFG within the Cluster of Excellence "Center for Advancing Electronics Dresden". The authors acknowledge the Center for Information Services and High Performance Computing (ZIH) at TU Dresden for computational resources.
    Publisher
    Wiley
    Journal
    Advanced Functional Materials
    DOI
    10.1002/adfm.201402334
    ae974a485f413a2113503eed53cd6c53
    10.1002/adfm.201402334
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; KAUST Solar Center (KSC)

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