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    N-heterocyclic carbene copper(I) catalysed N-methylation of amines using CO2

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    Type
    Article
    Authors
    Santoro, Orlando
    Lazreg, Faïma
    Minenkov, Yury cc
    Cavallo, Luigi cc
    Cazin, Catherine S. J. cc
    KAUST Department
    Chemical Science Program
    KAUST Catalysis Center (KCC)
    Physical Science and Engineering (PSE) Division
    Date
    2015
    Permanent link to this record
    http://hdl.handle.net/10754/592738
    
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    Abstract
    The N-methylation of amines using CO2 and PhSiH3 as source of CH3 was efficiently performed using a N-heterocyclic carbene copper(I) complex. The methodology was found compatible with aromatic and aliphatic primary and secondary amines. Synthetic and computational studies have been carried out to support the proposed reaction mechanism for this transformation.
    Citation
    N-heterocyclic carbene copper(I) catalysed N-methylation of amines using CO2 2015, 44 (41):18138 Dalton Trans.
    Publisher
    Royal Society of Chemistry (RSC)
    Journal
    Dalton Transactions
    DOI
    10.1039/C5DT03506F
    Additional Links
    http://xlink.rsc.org/?DOI=C5DT03506F
    ae974a485f413a2113503eed53cd6c53
    10.1039/C5DT03506F
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Chemical Science Program; KAUST Catalysis Center (KCC)

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