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dc.contributor.authorZhou, Lu
dc.contributor.authorLi, Lidong
dc.contributor.authorWei, Nini
dc.contributor.authorLi, Jun
dc.contributor.authorBasset, Jean-Marie
dc.date.accessioned2015-08-17T07:41:21Z
dc.date.available2015-08-17T07:41:21Z
dc.date.issued2015-07-16
dc.identifier.citationEffect of NiAl2O4 Formation on Ni/Al2O3 Stability during Dry Reforming of Methane 2015, 7 (16):2508 ChemCatChem
dc.identifier.issn18673880
dc.identifier.doi10.1002/cctc.201500379
dc.identifier.urihttp://hdl.handle.net/10754/567060
dc.description.abstractA series of alumina-supported Ni catalysts were prepared to examine their activity and carbon deposition during dry reforming of methane (DRM). With an increase in the final calcination temperature to T=900 °C to form exclusively NiAl2O4, a catalyst with strong metal–support interactions was obtained. During a long-term DRM reaction (of about t=100 h) at T=700 °C and with CH4/CO2=1:1, reduced Ni (from NiAl2O4) showed a high resistance to sintering and coking. The DRM kinetics behaviors of the catalysts calcined at different temperatures were also investigated. Carbon growth models were proposed to rationalize the different carbon morphologies observed on the catalysts.
dc.language.isoen
dc.publisherWiley
dc.relation.urlhttp://doi.wiley.com/10.1002/cctc.201500379
dc.rightsThis is the peer reviewed version of the following article: Zhou, L., Li, L., Wei, N., Li, J. and Basset, J.-M. (2015), Effect of NiAl2O4 Formation on Ni/Al2O3 Stability during Dry Reforming of Methane. ChemCatChem, 7: 2508–2516. doi: 10.1002/cctc.201500379, which has been published in final form at http://doi.wiley.com/10.1002/cctc.201500379. This article may be used for non-commercial purposes in accordance With Wiley Terms and Conditions for self-archiving.
dc.subjectcarbon
dc.subjectdry reforming
dc.subjectmethane
dc.subjectnickel
dc.subjectsupported catalysts
dc.titleEffect of NiAl2O4 Formation on Ni/Al2O3 Stability during Dry Reforming of Methane
dc.typeArticle
dc.contributor.departmentCatalysis for Energy Conversion (CatEC)
dc.contributor.departmentChemical Science Program
dc.contributor.departmentElectron Microscopy
dc.contributor.departmentKAUST Catalysis Center (KCC)
dc.contributor.departmentPhysical Science and Engineering (PSE) Division
dc.identifier.journalChemCatChem
dc.eprint.versionPost-print
dc.contributor.affiliationKing Abdullah University of Science and Technology (KAUST)
kaust.personZhou, Lu
kaust.personLi, Lidong
kaust.personTakanabe, Kazuhiro
kaust.personBasset, Jean-Marie
kaust.personWei, Nini
kaust.personLi, Jun
refterms.dateFOA2016-07-16T00:00:00Z
dc.date.published-online2015-07-16
dc.date.published-print2015-08-17


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