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    Catalytic conversion of methane: Carbon dioxide reforming and oxidative coupling

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    Type
    Article
    Authors
    Takanabe, Kazuhiro cc
    KAUST Department
    Biological and Environmental Sciences and Engineering (BESE) Division
    Chemical Science Program
    KAUST Catalysis Center (KCC)
    Date
    2012
    Permanent link to this record
    http://hdl.handle.net/10754/565958
    
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    Abstract
    Natural gas conversion remains one of the essential technologies for current energy needs. This review focuses on the mechanistic aspects of the development of efficient and durable catalysts for two reactions, carbon dioxide reforming and the oxidative coupling of methane. These two reactions have tremendous technological significance for practical application in industry. An understanding of the fundamental aspects and reaction mechanisms of the catalytic reactions reviewed in this study would support the design of industrial catalysts. CO 2 reforming of methane utilizes CO 2, which is often stored in large quantities, to convert as a reactant. Strategies to eliminate carbon deposition, which is the major problem associated with this reaction, are discussed. The oxidative coupling of methane directly produces ethylene in one reactor through a slightly exothermic reaction, potentially minimizing the capital cost of the natural gas conversion process. The focus of discussion in this review will be on the attainable yield of C 2 products by rigorous kinetic analyses.
    Citation
    Takanabe, K. (2012). Catalytic Conversion of Methane: Carbon Dioxide Reforming and Oxidative Coupling. Journal of the Japan Petroleum Institute, 55(1), 1–12. doi:10.1627/jpi.55.1
    Publisher
    Japan Petroleum Institute
    Journal
    Journal of the Japan Petroleum Institute
    DOI
    10.1627/jpi.55.1
    ae974a485f413a2113503eed53cd6c53
    10.1627/jpi.55.1
    Scopus Count
    Collections
    Articles; Biological and Environmental Science and Engineering (BESE) Division; Chemical Science Program; KAUST Catalysis Center (KCC)

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