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    Ordering effects in benzo[1,2-b:4,5-b']difuran-thieno[3,4-c]pyrrole-4,6- dione polymers with >7% solar cell efficiency

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    Type
    Article
    Authors
    Warnan, Julien
    Cabanetos, Clement
    El Labban, Abdulrahman cc
    Hansen, Michael Ryan
    Tassone, Christopher J.
    Toney, Michael F.
    Beaujuge, Pierre cc
    KAUST Department
    Biological and Environmental Sciences and Engineering (BESE) Division
    Chemical Science Program
    KAUST Solar Center (KSC)
    Material Science and Engineering Program
    Physical Science and Engineering (PSE) Division
    Date
    2014-05-15
    Online Publication Date
    2014-05-15
    Print Publication Date
    2014-07
    Permanent link to this record
    http://hdl.handle.net/10754/563549
    
    Metadata
    Show full item record
    Abstract
    Benzo[1,2-b:4,5-b']difuran-thieno[3,4-c]pyrrole-4,6-dione (PBDFTPD) polymers prepared by microwave-assisted synthesis can achieve power conversion efficiencies (PCEs) >7% in bulk-heterojunction solar cells with phenyl-C61/71-butyric acid methyl ester (PCBM). In "as-cast" PBDFTPD-based devices solution-processed without a small-molecule additive, high PCEs can be obtained in spite of the weak propensity of the polymers to self-assemble and form π-aggregates in thin films. © 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
    Citation
    Warnan, J., Cabanetos, C., Labban, A. E., Hansen, M. R., Tassone, C., Toney, M. F., & Beaujuge, P. M. (2014). Ordering Effects in Benzo[1,2-b:4,5-b′]difuran-thieno[3,4-c]pyrrole-4,6-dione Polymers with >7% Solar Cell Efficiency. Advanced Materials, 26(25), 4357–4362. doi:10.1002/adma.201305344
    Sponsors
    The authors acknowledge financial support under Baseline Research Funding from King Abdullah University of Science and Technology (KAUST). The authors thank KAUST Analytical Core Labs for mass spectrometry and elemental analyses, and Sandra Seywald (MPIP - Mainz, Germany) for SEC measurements. The authors thank the Advanced Imaging and Characterization Laboratories at KAUST for technical support. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource user facility, operated by Stanford University on behalf of the U.S. Department of Energy, Office of Basic Energy Sciences. MRH acknowledges financial support from the Villum Foundation under the Young Investigator Program.
    Publisher
    Wiley
    Journal
    Advanced Materials
    DOI
    10.1002/adma.201305344
    PubMed ID
    24829168
    ae974a485f413a2113503eed53cd6c53
    10.1002/adma.201305344
    Scopus Count
    Collections
    Articles; Biological and Environmental Science and Engineering (BESE) Division; Physical Science and Engineering (PSE) Division; Chemical Science Program; Material Science and Engineering Program; KAUST Solar Center (KSC)

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