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    Low temperature activation of methane over a zinc-exchanged heteropolyacid as an entry to its selective oxidation to methanol and acetic acid

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    Type
    Article
    Authors
    Patil, Umesh
    Saih, Youssef
    Abou-Hamad, Edy cc
    Hamieh, Ali Imad Ali cc
    Pelletier, Jeremie cc
    Basset, Jean-Marie cc
    KAUST Department
    Ali I. Al-Naimi Petroleum Engineering Research Center (ANPERC)
    Chemical Science Program
    KAUST Catalysis Center (KCC)
    Physical Science and Engineering (PSE) Division
    Date
    2014
    Permanent link to this record
    http://hdl.handle.net/10754/563243
    
    Metadata
    Show full item record
    Abstract
    A Zn-exchanged heteropolyacid supported onto silica (Zn-HPW/SiO2) activates methane at 25 °C into Zn-methyl. At higher temperatures and with CH4/O2 or CH4/CO2, it gives methanol and acetic acid respectively. This journal is
    Citation
    Patil, U., Saih, Y., Abou-Hamad, E., Hamieh, A., Pelletier, J. D. A., & Basset, J. M. (2014). Low temperature activation of methane over a zinc-exchanged heteropolyacid as an entry to its selective oxidation to methanol and acetic acid. Chem. Commun., 50(82), 12348–12351. doi:10.1039/c4cc04950k
    Sponsors
    We gratefully acknowledge King Abdullah University of Science and Technology (KAUST) and Saudi Basic Industries Corporation (SABIC) for financial support.
    Publisher
    Royal Society of Chemistry (RSC)
    Journal
    Chem. Commun.
    DOI
    10.1039/c4cc04950k
    PubMed ID
    25182752
    ae974a485f413a2113503eed53cd6c53
    10.1039/c4cc04950k
    Scopus Count
    Collections
    Articles; Ali I. Al-Naimi Petroleum Engineering Research Center (ANPERC); Physical Science and Engineering (PSE) Division; Chemical Science Program; KAUST Catalysis Center (KCC)

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