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    [(≡SiO)TaV (=CH2)Cl2], the first tantalum methylidene species prepared and identified on the silica surface

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    Type
    Article
    Authors
    Chen, Yin
    Callens, Emmanuel cc
    Abou-Hamad, Edy cc
    Basset, Jean-Marie cc
    KAUST Department
    Chemical Science Program
    KAUST Catalysis Center (KCC)
    KAUST Solar Center (KSC)
    Physical Science and Engineering (PSE) Division
    Date
    2013-11
    Permanent link to this record
    http://hdl.handle.net/10754/563064
    
    Metadata
    Show full item record
    Abstract
    A novel surface tantalum methylidene [(≡SiO)TaV (=CH 2)Cl2] was obtained via thermal decomposition of the well-defined surface species [(≡SiO)TaVCl2Me 2]. This first surface tantalum methylidene ever synthesized has been fully characterized and the kinetics of the a-hydrogen abstraction reaction has also been investigated in the heterogeneous system. © 2013 Elsevier B.V. All rights reserved.
    Citation
    Chen, Y., Callens, E., Abou-hamad, E., & Basset, J.-M. (2013). [(SiO)TaV(CH2)Cl2], the first tantalum methylidene species prepared and identified on the silica surface. Journal of Organometallic Chemistry, 744, 3–6. doi:10.1016/j.jorganchem.2013.04.050
    Sponsors
    We thanks KAUST for the financial support and YC gratefully acknowledges generous donation from SABIC.
    Publisher
    Elsevier BV
    Journal
    Journal of Organometallic Chemistry
    DOI
    10.1016/j.jorganchem.2013.04.050
    ae974a485f413a2113503eed53cd6c53
    10.1016/j.jorganchem.2013.04.050
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Chemical Science Program; KAUST Catalysis Center (KCC); KAUST Solar Center (KSC)

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