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    Post-synthetic modification of porphyrin-encapsulating metal-organic materials by cooperative addition of inorganic salts to enhance CO 2/CH 4 selectivity

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    Type
    Article
    Authors
    Zhang, Zhenjie
    Gao, Wenyang
    Wojtas, Łukasz
    Ma, Shengqian
    Eddaoudi, Mohamed cc
    Zaworotko, Michael J.
    KAUST Department
    Advanced Membranes and Porous Materials Research Center
    Biological and Environmental Sciences and Engineering (BESE) Division
    Chemical Science Program
    Functional Materials Design, Discovery and Development (FMD3)
    Physical Science and Engineering (PSE) Division
    Date
    2012-08-21
    Online Publication Date
    2012-08-21
    Print Publication Date
    2012-09-10
    Permanent link to this record
    http://hdl.handle.net/10754/562279
    
    Metadata
    Show full item record
    Abstract
    Keeping MOM: Reaction of biphenyl-3,4',5-tricarboxylate and Cd(NO 3) 2 in the presence of meso-tetra(N-methyl-4-pyridyl) porphine tetratosylate afforded porph@MOM-11, a microporous metal-organic material (MOM) that encapsulates cationic porphyrins and solvent in alternating open channels. Porph@MOM-11 has cation and anion binding sites that facilitate cooperative addition of inorganic salts (such as M +Cl -) in a stoichiometric fashion. © 2012 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.
    Citation
    Zhang, Z., Gao, W.-Y., Wojtas, L., Ma, S., Eddaoudi, M., & Zaworotko, M. J. (2012). Post-Synthetic Modification of Porphyrin-Encapsulating Metal-Organic Materials by Cooperative Addition of Inorganic Salts to Enhance CO2/CH4Selectivity. Angewandte Chemie International Edition, 51(37), 9330–9334. doi:10.1002/anie.201203594
    Sponsors
    This work is supported by King Abdullah University of Science and Technology (FIC/2010/06). The microcrystal diffraction of porph(Cl<SUP>-</SUP>)@MOM-11(Mn<SUP>2+</SUP>) was carried at the Advanced Photon Source on beamline 15ID-B at ChemMatCARS Sector 15 (NSF/CHE-0822838 and DE-AC02-06CH11357).
    Publisher
    Wiley
    Journal
    Angewandte Chemie
    DOI
    10.1002/anie.201203594
    Relations
    Is Supplemented By:
    • [Dataset]
      Zhang, Z., Gao, W.-Y., Wojtas, L., Ma, S., Eddaoudi, M., & Zaworotko, M. J. (2013). CCDC 878570: Experimental Crystal Structure Determination [Data set]. Cambridge Crystallographic Data Centre. https://doi.org/10.5517/ccyh6zl. DOI: 10.5517/ccyh6zl HANDLE: 10754/624700
    • [Dataset]
      Zhang, Z., Gao, W.-Y., Wojtas, L., Ma, S., Eddaoudi, M., & Zaworotko, M. J. (2013). CCDC 878571: Experimental Crystal Structure Determination [Data set]. Cambridge Crystallographic Data Centre. https://doi.org/10.5517/ccyh70n. DOI: 10.5517/ccyh70n HANDLE: 10754/624701
    • [Dataset]
      Zhang, Z., Gao, W.-Y., Wojtas, L., Ma, S., Eddaoudi, M., & Zaworotko, M. J. (2013). CCDC 878572: Experimental Crystal Structure Determination [Data set]. Cambridge Crystallographic Data Centre. https://doi.org/10.5517/ccyh71p. DOI: 10.5517/ccyh71p HANDLE: 10754/624702
    • [Dataset]
      Zhang, Z., Gao, W.-Y., Wojtas, L., Ma, S., Eddaoudi, M., & Zaworotko, M. J. (2013). CCDC 878573: Experimental Crystal Structure Determination [Data set]. Cambridge Crystallographic Data Centre. https://doi.org/10.5517/ccyh72q. DOI: 10.5517/ccyh72q HANDLE: 10754/624703
    • [Dataset]
      Zhang, Z., Gao, W.-Y., Wojtas, L., Ma, S., Eddaoudi, M., & Zaworotko, M. J. (2013). CCDC 878574: Experimental Crystal Structure Determination [Data set]. Cambridge Crystallographic Data Centre. https://doi.org/10.5517/ccyh73r. DOI: 10.5517/ccyh73r HANDLE: 10754/624704
    ae974a485f413a2113503eed53cd6c53
    10.1002/anie.201203594
    Scopus Count
    Collections
    Articles; Biological and Environmental Science and Engineering (BESE) Division; Advanced Membranes and Porous Materials Research Center; Physical Science and Engineering (PSE) Division; Functional Materials Design, Discovery and Development (FMD3); Chemical Science Program

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