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    Tetrakis(4-tert-butylphenyl) substituted and fused quinoidal porphyrins

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    Type
    Article
    Authors
    Zeng, Wangdong
    Lee, Byungsun
    Sung, Youngmo
    Huang, Kuo-Wei cc
    Li, Yuan
    Kim, Dongho
    Wu, Jishan
    KAUST Department
    Biological and Environmental Sciences and Engineering (BESE) Division
    Chemical Science Program
    Homogeneous Catalysis Laboratory (HCL)
    KAUST Catalysis Center (KCC)
    Physical Science and Engineering (PSE) Division
    Date
    2012
    Permanent link to this record
    http://hdl.handle.net/10754/562008
    
    Metadata
    Show full item record
    Abstract
    4-tert-Butylphenyl-substituted and fused quinoidal porphyrins 1 and 2 are prepared for the first time. They show (1) intense one-photon absorption in the far-red/near-infrared region, (2) enhanced two-photon absorption compared with aromatic porphyrin monomers, and (3) amphoteric redox behavior. Their geometry and electronic structure are studied by DFT calculations. This journal is © 2012 The Royal Society of Chemistry.
    Citation
    Zeng, W., Lee, B. S., Sung, Y. M., Huang, K.-W., Li, Y., Kim, D., & Wu, J. (2012). Tetrakis(4-tert-butylphenyl) substituted and fused quinoidal porphyrins. Chemical Communications, 48(62), 7684. doi:10.1039/c2cc33728b
    Sponsors
    J. W. acknowledges the financial support from the BMRC-NMRC grant (no. 10/1/21/19/642), MOE Tier 2 grant (MOE2011-T2-2-130) and IMRE Core Funding (IMRE/10-1P0509). The work at Yonsei Univ. was supported by WCU (World Class University) programs (R32-2010-10217-0) and an AFSOR/APARD grant (no. FA2386-09-1-4092). K.-W. H. acknowledges the financial support from KAUST.
    Publisher
    Royal Society of Chemistry (RSC)
    Journal
    Chemical Communications
    DOI
    10.1039/c2cc33728b
    ae974a485f413a2113503eed53cd6c53
    10.1039/c2cc33728b
    Scopus Count
    Collections
    Articles; Biological and Environmental Science and Engineering (BESE) Division; Physical Science and Engineering (PSE) Division; Chemical Science Program; KAUST Catalysis Center (KCC)

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