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    Experimental and first-principles study of ferromagnetism in Mn-doped zinc stannate nanowires

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    Type
    Article
    Authors
    Deng, Rui
    Zhou, Hang
    Li, Yong-Feng
    Wu, Tao cc
    Yao, Bin
    Qin, Jie-Ming
    Wan, Yu-Chun
    Jiang, Da-Yong
    Liang, Qing-Cheng
    Liu, Lei
    KAUST Department
    KAUST Solar Center (KSC)
    Laboratory of Nano Oxides for Sustainable Energy
    Material Science and Engineering Program
    Physical Science and Engineering (PSE) Division
    Date
    2013-07-17
    Online Publication Date
    2013-07-17
    Print Publication Date
    2013-07-21
    Permanent link to this record
    http://hdl.handle.net/10754/552529
    
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    Abstract
    Room temperature ferromagnetism was observed in Mn-doped zinc stannate (ZTO:Mn) nanowires, which were prepared by chemical vapor transport. Structural and magnetic properties and Mn chemical states of ZTO:Mn nanowires were investigated by X-ray diffraction, superconducting quantum interference device (SQUID) magnetometry and X-ray photoelectron spectroscopy. Manganese predominantly existed as Mn2+ and substituted for Zn (Mn Zn) in ZTO:Mn. This conclusion was supported by first-principles calculations. MnZn in ZTO:Mn had a lower formation energy than that of Mn substituted for Sn (MnSn). The nearest neighbor MnZn in ZTO stabilized ferromagnetic coupling. This observation supported the experimental results. © 2013 AIP Publishing LLC.
    Citation
    Experimental and first-principles study of ferromagnetism in Mn-doped zinc stannate nanowires 2013, 114 (3):033910 Journal of Applied Physics
    Publisher
    AIP Publishing
    Journal
    Journal of Applied Physics
    DOI
    10.1063/1.4815884
    Additional Links
    http://scitation.aip.org/content/aip/journal/jap/114/3/10.1063/1.4815884
    ae974a485f413a2113503eed53cd6c53
    10.1063/1.4815884
    Scopus Count
    Collections
    Articles; Physical Science and Engineering (PSE) Division; Material Science and Engineering Program; KAUST Solar Center (KSC)

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