Heterogeneous shear elasticity of glasses: The origin of the boson peak
KAUST DepartmentPRIMALIGHT Research Group
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AbstractThe local elasticity of glasses is known to be inhomogeneous on a microscopic scale compared to that of crystalline materials. Their vibrational spectrum strongly deviates from that expected from Debye's elasticity theory: The density of states deviates from Debye's law, the sound velocity shows a negative dispersion in the boson-peak frequency regime and there is a strong increase of the sound attenuation near the boson-peak frequency. By comparing a mean-field theory of shear-elastic heterogeneity with a large-scale simulation of a soft-sphere glass we demonstrate that the observed anomalies in glasses are caused by elastic heterogeneity. By observing that the macroscopic bulk modulus is frequency independent we show that the boson-peak-related vibrational anomalies are predominantly due to the spatially fluctuating microscopic shear stresses. It is demonstrated that the boson-peak arises from the steep increase of the sound attenuation at a frequency which marks the transition from wave-like excitations to disorder-dominated ones.
CitationMarruzzo A, Schirmacher W, Fratalocchi A, Ruocco G (2013) Heterogeneous shear elasticity of glasses: the origin of the boson peak. Sci Rep 3. doi:10.1038/srep01407.
PublisherNature Publishing Group
PubMed Central IDPMC3591752
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