High-Purity Hybrid Organolead Halide Perovskite Nanoparticles Obtained by Pulsed-Laser Irradiation in Liquid

Handle URI:
http://hdl.handle.net/10754/622662
Title:
High-Purity Hybrid Organolead Halide Perovskite Nanoparticles Obtained by Pulsed-Laser Irradiation in Liquid
Authors:
Amendola, Vincenzo; Fortunati, Ilaria; Marega, Carla; Abdelhady, Ahmed L.; Saidaminov, Makhsud I. ( 0000-0002-3850-666X ) ; Bakr, Osman M. ( 0000-0002-3428-1002 )
Abstract:
Nanoparticles of hybrid organic-inorganic perovskites have attracted a great deal of attention due to their variety of optoelectronic properties, their low cost, and their easier integration into devices with complex geometry, compared with microcrystalline, thin-film, or bulk metal halides. Here we present a novel one-step synthesis of organolead bromide perovskite nanocrystals based on pulsed-laser irradiation in a liquid environment (PLIL). Starting from a bulk CHNHPbBr crystal, our PLIL procedure does not involve the use of high-boiling-point polar solvents or templating agents, and runs at room temperature. The resulting nanoparticles are characterized by high crystallinity and are completely free of any microscopic product or organic coating layer. We also demonstrate the straightforward inclusion of laser-generated perovskite nanocrystals in a polymeric matrix to form a nanocomposite with single- and two-photon luminescence properties.
KAUST Department:
Physical Sciences and Engineering (PSE) Division
Citation:
Amendola V, Fortunati I, Marega C, Abdelhady AL, Saidaminov MI, et al. (2016) High-Purity Hybrid Organolead Halide Perovskite Nanoparticles Obtained by Pulsed-Laser Irradiation in Liquid. ChemPhysChem. Available: http://dx.doi.org/10.1002/cphc.201600863.
Publisher:
Wiley-Blackwell
Journal:
ChemPhysChem
Issue Date:
17-Nov-2016
DOI:
10.1002/cphc.201600863
Type:
Article
ISSN:
1439-4235
Sponsors:
The authors thank Stefano Scaramuzza for support with LAL. Financial support from the University of Padova (PRAT no. CPDA114097/11) is gratefully acknowledged.
Additional Links:
http://onlinelibrary.wiley.com/doi/10.1002/cphc.201600863/full
Appears in Collections:
Articles; Physical Sciences and Engineering (PSE) Division

Full metadata record

DC FieldValue Language
dc.contributor.authorAmendola, Vincenzoen
dc.contributor.authorFortunati, Ilariaen
dc.contributor.authorMarega, Carlaen
dc.contributor.authorAbdelhady, Ahmed L.en
dc.contributor.authorSaidaminov, Makhsud I.en
dc.contributor.authorBakr, Osman M.en
dc.date.accessioned2017-01-09T11:52:22Z-
dc.date.available2017-01-09T11:52:22Z-
dc.date.issued2016-11-17en
dc.identifier.citationAmendola V, Fortunati I, Marega C, Abdelhady AL, Saidaminov MI, et al. (2016) High-Purity Hybrid Organolead Halide Perovskite Nanoparticles Obtained by Pulsed-Laser Irradiation in Liquid. ChemPhysChem. Available: http://dx.doi.org/10.1002/cphc.201600863.en
dc.identifier.issn1439-4235en
dc.identifier.doi10.1002/cphc.201600863en
dc.identifier.urihttp://hdl.handle.net/10754/622662-
dc.description.abstractNanoparticles of hybrid organic-inorganic perovskites have attracted a great deal of attention due to their variety of optoelectronic properties, their low cost, and their easier integration into devices with complex geometry, compared with microcrystalline, thin-film, or bulk metal halides. Here we present a novel one-step synthesis of organolead bromide perovskite nanocrystals based on pulsed-laser irradiation in a liquid environment (PLIL). Starting from a bulk CHNHPbBr crystal, our PLIL procedure does not involve the use of high-boiling-point polar solvents or templating agents, and runs at room temperature. The resulting nanoparticles are characterized by high crystallinity and are completely free of any microscopic product or organic coating layer. We also demonstrate the straightforward inclusion of laser-generated perovskite nanocrystals in a polymeric matrix to form a nanocomposite with single- and two-photon luminescence properties.en
dc.description.sponsorshipThe authors thank Stefano Scaramuzza for support with LAL. Financial support from the University of Padova (PRAT no. CPDA114097/11) is gratefully acknowledged.en
dc.publisherWiley-Blackwellen
dc.relation.urlhttp://onlinelibrary.wiley.com/doi/10.1002/cphc.201600863/fullen
dc.subjectLaser chemistryen
dc.subjectMetal halidesen
dc.subjectNanoparticlesen
dc.subjectOrganoleaden
dc.subjectPerovskite phasesen
dc.titleHigh-Purity Hybrid Organolead Halide Perovskite Nanoparticles Obtained by Pulsed-Laser Irradiation in Liquiden
dc.typeArticleen
dc.contributor.departmentPhysical Sciences and Engineering (PSE) Divisionen
dc.identifier.journalChemPhysChemen
dc.contributor.institutionDepartment of Chemical Sciences; University of Padova; via Marzolo 1 35131 Padova Italyen
kaust.authorAbdelhady, Ahmed L.en
kaust.authorSaidaminov, Makhsud I.en
kaust.authorBakr, Osman M.en
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