Handle URI:
http://hdl.handle.net/10754/599077
Title:
Onsager Reciprocity in Premelting Solids
Authors:
Peppin, S. S. L.; Spannuth, M. J.; Wettlaufer, J. S.
Abstract:
The diffusive motion of foreign particles dispersed in a premelting solid is analyzed within the framework of irreversible thermodynamics. We determine the mass diffusion coefficient, thermal diffusion coefficient and Soret coefficient of the particles in the dilute limit, and find good agreement with experimental data. In contrast to liquid suspensions, the unique nature of premelting solids allows us to derive an expression for the Dufour coefficient and independently verify the Onsager reciprocal relation coupling diffusion to the flow of heat. © 2009 Springer Science+Business Media, LLC.
Citation:
Peppin SSL, Spannuth MJ, Wettlaufer JS (2009) Onsager Reciprocity in Premelting Solids. J Stat Phys 134: 701–708. Available: http://dx.doi.org/10.1007/s10955-009-9699-z.
Publisher:
Springer Nature
Journal:
Journal of Statistical Physics
KAUST Grant Number:
KUK-C1-013-04
Issue Date:
Feb-2009
DOI:
10.1007/s10955-009-9699-z
Type:
Article
ISSN:
0022-4715; 1572-9613
Sponsors:
This research was supported by the Department of Energy (DE-FG02-05ER15741) and by the U. S. National Science Foundation (OPP0440841). S. S. L. P. acknowledges support from the King Abdullah University of Science and Technology (KAUST), Award No. KUK-C1-013-04. M. J. S. acknowledges support from a U. S. National Science Foundation Graduate Research Fellowship. J. S. W. is grateful for support from the Wenner-Gren Foundation, the Royal Institute of Technology and NORDITA all in Stockholm.
Appears in Collections:
Publications Acknowledging KAUST Support

Full metadata record

DC FieldValue Language
dc.contributor.authorPeppin, S. S. L.en
dc.contributor.authorSpannuth, M. J.en
dc.contributor.authorWettlaufer, J. S.en
dc.date.accessioned2016-02-25T13:52:26Zen
dc.date.available2016-02-25T13:52:26Zen
dc.date.issued2009-02en
dc.identifier.citationPeppin SSL, Spannuth MJ, Wettlaufer JS (2009) Onsager Reciprocity in Premelting Solids. J Stat Phys 134: 701–708. Available: http://dx.doi.org/10.1007/s10955-009-9699-z.en
dc.identifier.issn0022-4715en
dc.identifier.issn1572-9613en
dc.identifier.doi10.1007/s10955-009-9699-zen
dc.identifier.urihttp://hdl.handle.net/10754/599077en
dc.description.abstractThe diffusive motion of foreign particles dispersed in a premelting solid is analyzed within the framework of irreversible thermodynamics. We determine the mass diffusion coefficient, thermal diffusion coefficient and Soret coefficient of the particles in the dilute limit, and find good agreement with experimental data. In contrast to liquid suspensions, the unique nature of premelting solids allows us to derive an expression for the Dufour coefficient and independently verify the Onsager reciprocal relation coupling diffusion to the flow of heat. © 2009 Springer Science+Business Media, LLC.en
dc.description.sponsorshipThis research was supported by the Department of Energy (DE-FG02-05ER15741) and by the U. S. National Science Foundation (OPP0440841). S. S. L. P. acknowledges support from the King Abdullah University of Science and Technology (KAUST), Award No. KUK-C1-013-04. M. J. S. acknowledges support from a U. S. National Science Foundation Graduate Research Fellowship. J. S. W. is grateful for support from the Wenner-Gren Foundation, the Royal Institute of Technology and NORDITA all in Stockholm.en
dc.publisherSpringer Natureen
dc.subjectColloidsen
dc.subjectDiffusionen
dc.subjectDufour effecten
dc.subjectPremeltingen
dc.subjectReciprocityen
dc.subjectSoret effecten
dc.subjectSurface phase transitionsen
dc.titleOnsager Reciprocity in Premelting Solidsen
dc.typeArticleen
dc.identifier.journalJournal of Statistical Physicsen
dc.contributor.institutionYale University, New Haven, United Statesen
dc.contributor.institutionUniversity of Oxford, Oxford, United Kingdomen
dc.contributor.institutionNordisk Institut for Teoretisk Atomtysik, Stockholm, Swedenen
kaust.grant.numberKUK-C1-013-04en
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